Reconstruction of uranium and plutonium isotopic signatures in sediment accumulated in the Mano Dam reservoir, Japan, before and after the Fukushima nuclear accident

Hugo Jaegler (1) , Fabien Pointurier (2) , Silvia Diez-Fernández (3) , Alkiviadis Gourgiotis (4) , Hélène Isnard (3) , Seiji Hayashi (5) , Hideki Tsuji (5) , Yuichi Onda (6) , Amelie Hubert (2) , J. Patrick Laceby (1) , O. Evrard (1, 7)

1 LSCE - Laboratoire des Sciences du Climat et de l'Environnement [Gif-sur-Yvette]
2 CEA/DAM
3 CEA/DEN
4 IRSN/PSE-ENV/SEDRE/LELI - Laboratoire de recherche sur le devenir des pollutions de sites radioactifs
5 National Institute for Environmental Science [Fukushima]
6 Center for Research in Isotopes and Environmental Dynamics
7 ESTIMR - Extrèmes : Statistiques, Impacts et Régionalisation

The Fukushima Dai-ichi Nuclear Power Plant (FDNPP) accident in Japan resulted in a major release of radionuclides into the environment. Compared to other radionuclides, few studies have investigated the emission of actinides. Accordingly, this research investigates the Pu composition in soil samples collected in paddy fields before and after the accident. Furthermore, the vertical distributions of Pu and U isotopic signatures, along with 137Cs activities, were measured in a sediment core collected in the Mano Dam reservoir, in the Fukushima Prefecture. Changes in the relative contributions of the major actinide sources (global fallout or FDNPP derived fallout) were investigated in sediment deposited in the reservoir. The distinct peak observed for all Pu isotope ratios (240Pu/239Pu, 241Pu/239Pu and 242Pu/239Pu) and for 137Cs concentrations in the sediment core was attributed to the Fukushima fallout, and coincided with the maximum atomic contribution of only 4.8 ± 1.0 % of Pu from the FDNPP. Furthermore, 236U/238U ratios measured in the sediment core remained close to the global fallout signature indicating there was likely no U from the FDNPP accident in the sediment core. More research is required on the environmental dynamics of trace actinides in landscapes closer to the FDNPP where there are likely to be greater abundances of FDNPP-derived Pu and U.

Domaines: Sciences de l'environnement

Hugo Jaegler, Fabien Pointurier, Silvia Diez-Fernández, Alkiviadis Gourgiotis, Hélène Isnard, et al.. Reconstruction of uranium and plutonium isotopic signatures in sediment accumulated in the Mano Dam reservoir, Japan, before and after the Fukushima nuclear accident. Chemosphere, 2019, 225, pp.849-858. ⟨10.1016/j.chemosphere.2019.03.064⟩. ⟨hal-02336278⟩