Towards enabling femtosecond helicity-dependent spectroscopy with high-harmonic sources

Abstract : Recent advances in high-harmonic generation gave rise to soft X-ray pulses with higher intensity, shorter duration and higher photon energy. One of the remaining shortages of this source is its restriction to linear polarization, since the yield of generation of elliptically polarized high harmonics has been low so far. We here show how this limitation is overcome by using a cross-polarized two-colour laser field. With this simple technique, we reach high degrees of ellipticity (up to 75%) with efficiencies similar to classically generated linearly polarized harmonics. To demonstrate these features and to prove the capacity of our source for applications, we measure the X-ray magnetic circular dichroism (XMCD) effect of nickel at the M2,3 absorption edge around 67 eV. There results open up the way towards femtosecond time-resolved experiments using high harmonics exploiting the powerful element-sensitive XMCD effect and resolving the ultrafast magnetization dynamics of individual components in complex materials.
Complete list of metadatas

https://hal.archives-ouvertes.fr/hal-01164378
Contributor : Victor Malka <>
Submitted on : Tuesday, June 16, 2015 - 5:08:01 PM
Last modification on : Wednesday, September 4, 2019 - 5:36:03 PM

Links full text

Identifiers

Citation

Guillaume Lambert, B. Vodungbo, J. Gautier, B. Mahieu, Victor Malka, et al.. Towards enabling femtosecond helicity-dependent spectroscopy with high-harmonic sources. Nature Communications, Nature Publishing Group, 2015, 6, pp.6167. ⟨10.1038/ncomms7167⟩. ⟨hal-01164378⟩

Share

Metrics

Record views

361