Structure of molecular packing probed by polarization-resolved nonlinear four-wave mixing and coherent anti-Stokes Raman-scattering microscopy

Abstract : We report a method that is able to provide refined structural information on molecular packing in biomolecular assemblies using polarization-resolved four-wavemixing and coherent anti-Stokes Raman-scattering microscopy. These third-order nonlinear processes allow quantifying high orders of symmetry which are exploited here to reveal a high level of detail in the angular disorder behavior at the molecular scale in lipid membranes.
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F.-Z. Bioud, P. Gasecka, P. Ferrand, H. Rigneault, J. Duboisset, et al.. Structure of molecular packing probed by polarization-resolved nonlinear four-wave mixing and coherent anti-Stokes Raman-scattering microscopy. Physical Review A, American Physical Society, 2014, 89 (1), pp.013836. ⟨10.1103/PhysRevA.89.013836⟩. ⟨hal-00937566⟩

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