The importance of the beta spectrum calculation for accurate activity determination of 63 Ni by means of liquid scintillation counting

Karsten Kossert (1) , Xavier Mougeot (2)

1 PTB - Physikalisch-Technische Bundesanstalt [Braunschweig]
2 LNHB (CEA, LIST) - Laboratoire National Henri Becquerel (CEA, LIST)

The activity concentration of a Ni-63 solution was determined by means of two liquid scintillation counting techniques: the TDCR method and the CIEMAT/NIST efficiency tracing technique. The results of both methods are in excellent agreement, provided that the Ni-63 beta spectrum calculation accounts for the atomic exchange effect. Thus, new beta spectrum calculations resolve a discrepancy that has been found in previous analyses. The influence of the computed beta spectrum on the final uncertainty of the activity concentration is discussed.

Mots clés: 63Ni beta spectrum; Exchange effect; Liquid scintillation counting; TDCR; standardization

Domaines: Physique Nucléaire Expérimentale [nucl-ex]; Physique Nucléaire Théorique [nucl-th]

Karsten Kossert, Xavier Mougeot. The importance of the beta spectrum calculation for accurate activity determination of 63 Ni by means of liquid scintillation counting. Applied Radiation and Isotopes, 2015, 101, pp.40 - 43. ⟨10.1016/j.apradiso.2015.03.017⟩. ⟨hal-01864273⟩