Global chemical weather forecasts for field campaign planning: predictions and observations of large-scale features during MINOS, CONTRACE, and INDOEX

M. G. Lawrence (1) , P. J. Rasch (2) , R. von Kuhlmann (1) , J. Williams (1) , H. Fischer (1) , M. de Reus (1) , J. Lelieveld (1) , P. J. Crutzen (1) , M. Schultz (3) , P. Stier (3) , H. Huntrieser (4) , J. Heland (4) , A. Stohl (5) , C. Forster (5) , H. Elbern (6) , H. Jakobs (6) , R. R. Dickerson (7)

1 MPIC - Max-Planck-Institut für Chemie
2 NCAR - National Center for Atmospheric Research [Boulder]
3 MPI-M - Max-Planck-Institut für Meteorologie
4 IPA - DLR Institut für Physik der Atmosphäre = DLR Institute of Atmospheric Physics
5 Institute of Bioinformatics and Systems Biology [München]
6 Institut für Geophysik und Meteorologie [Braunschweig]
7 Department of Meteorology

The first global tropospheric forecasts of O₃ and its precursors have been used in the daily flight planning of field measurement campaigns. The 3-D chemistry-transport model MATCH-MPIC is driven by meteorological data from a weather center (NCEP) to produce daily 3-day forecasts of the global distributions of O₃ and related gases, as well as regional CO tracers. This paper describes the forecast system and its use in three field campaigns, MINOS, CONTRACE and INDOEX. An overview is given of the forecasts by MATCH-MPIC and by three other chemical weather forecast models (EURAD, ECHAM, and FLEXPART), focusing on O₃ and CO. Total CO and regional CO tracers were found to be the most valuable gases for flight planning, due to their relatively well-defined anthropogenic source regions and lifetimes of one to a few months. CO was in good agreement with the observations on nearly all the flights (generally r > 0.7, RMS < 20%). In every case in which the chemical weather forecasts were primarily responsible for the flight plans, the targeted features were observed. Two forecasted phenomena are discussed in detail: outflow from Asia observed in the Mediterranean upper troposphere during MINOS, and outflow from North America observed in the middle troposphere over northern Europe during CONTRACE. It is shown that although such pollution plumes occur repeatedly during the months around the campaigns, their frequency is sufficiently low (~10--30% of the time) that global chemical weather forecasts are important for enabling them to be observed during limited-duration field campaigns. The MATCH-MPIC chemical weather forecasts, including an interface for making customized figures from the output, are available for community use via http://www.mpch-mainz.mpg.de/~lawrence/forecasts.html .

Domaines: Océan, Atmosphère

M. G. Lawrence, P. J. Rasch, R. von Kuhlmann, J. Williams, H. Fischer, et al.. Global chemical weather forecasts for field campaign planning: predictions and observations of large-scale features during MINOS, CONTRACE, and INDOEX. Atmospheric Chemistry and Physics Discussions, 2002, 2 (5), pp.1545-1597. ⟨hal-00300919⟩