Laser pulse duration effects in Xe2+ ions induced by multiphoton absorption at 0.53 μm

A. L'Huillier , L.A. Lompre , G. Mainfray , C. Manus

Xe2+ ions can easily be formed by multiphoton absorption in Xe atoms at 0.53 μm. At low laser intensities, a laser-Xe atom interaction takes place which generates Xe2+ ions through a 15-photon absorption from Xe atoms. At higher intensities, a laser-Xe+ ion interaction takes place, generating Xe2+ ions through a 10-photon absorption from the Xe+ ion in its ground state. The former process is very sensitive to the laser pulse duration in the 5-200 ps range used here. As an example, the number of Xe2+ ions is increased by a factor of 30 when the pulse duration is decreased from 30 to 5 ps. The laser intensity at which this occurs is approximately 1012 W . cm- 2. A kinetic model is developed which is based on the rate equations describing the evolution of populations of Xe atoms, Xe + and Xe2+ ions. The result is that the ratio of the number of Xe2+ to Xe+ ions varies with the pulse duration τ as τ-3/2.

Keywords: ionisation of atoms; multiphoton spectra; photoionisation; xenon

Domains: Physics archives

A. L'Huillier, L.A. Lompre, G. Mainfray, C. Manus. Laser pulse duration effects in Xe2+ ions induced by multiphoton absorption at 0.53 μm. Journal de Physique, 1983, 44 (11), pp.1247-1255. ⟨10.1051/jphys:0198300440110124700⟩. ⟨jpa-00209709⟩