Measurements in a highly polluted Asian mega city: observations of aerosol number size distribution, modal parameters and nucleation events

P. Mönkkönen (1) , I. K. Koponen (1) , K. E. J. Lehtinen (1) , K. Hämeri (1, 2) , R. Uma (3) , M. Kulmala (1)

1 Helsingin yliopisto = Helsingfors universitet = University of Helsinki
2 Unit of Excellence for Psychosocial Factors
3 The Energy and Resources Institute (TERI)

Diurnal variation of number size distribution (particle size 3?800 nm) and modal parameters (geometric standard deviation, geometric mean diameter and modal aerosol particle concentration) in a highly polluted urban environment was investigated during October and November 2002 in New Delhi, India. Continuous monitoring for more than two weeks with the time resolution of 10 min was conducted using a Differential Mobility Particle Sizer (twin DMPS). The results indicated clear increase in Aitken mode (25?100 nm) particles during traffic peak hours, but towards the evenings there were more Aitken mode particles compared to the mornings. Also high concentrations of accumulation mode particles (>100 nm) were detected in the evenings only. In the evenings, biomass/refuse burning and cooking are possible sources beside the traffic. We have also shown that nucleation events are possible in this kind of atmosphere even though as clear nucleation events as observed in rural sites could not be detected. The formation rate of 3 nm particles (J3) of the observed events varied from 3.3 to 13.9 cm^?3s^?1 and the growth rate varied from 11.6 to 18.1 nmh^?1 showing rapid growth and high formation rate, which seems to be typical in urban areas.

Domaines: Océan, Atmosphère

P. Mönkkönen, I. K. Koponen, K. E. J. Lehtinen, K. Hämeri, R. Uma, et al.. Measurements in a highly polluted Asian mega city: observations of aerosol number size distribution, modal parameters and nucleation events. Atmospheric Chemistry and Physics Discussions, 2004, 4 (5), pp.5407-5431. ⟨hal-00301429⟩