Identification of damage mechanisms in concrete under high level creep by the acoustic emission technique

Many researchers have proposed hypoth-eses concerning the physical mechanisms that govern creep and among them the development of microcracks is well recognized. For high load levels, microcracking may initiates at the moment of load application and begins to grow to form a time-dependent crack path. An experimental investigation is proposed here in order to provide interesting insight into the coupling between creep and damage with specimens loaded in ﬂexure. The acoustic emission (AE) technique is used as a tool to provide information on the pertinence of the physical hypothesis that microcracks appear during creep. An original test is performed to accelerate the creep phenomenon by submitting concrete beams to desiccation after a basic creep period. The results show a good proportionality between the creep deformation and the AE activity and thus the efﬁciency of acoustic measurements for the estimation of the state of damage. In addition, an unsupervised pattern recognition analysis is used as a tool for the classiﬁcation of the monitored AE signatures. The cluster analysis shows two clusters during basic creep and three clusters during desiccation creep indicating different damage mechanisms.


Introduction
Concrete structures are susceptible to degradation due to delayed strains which has an impact on their safety margin and life time, especially when they are subjected to high loading level. Numerous contradictory theories have been put forward over the years to assess the creep behaviour of concrete. Since no single mechanism can account for all the observed phenomena, several major real mechanisms can be distinguished and it is commonly accepted that a combination of these mechanisms acts together. Usually, creep mechanisms are associated with the hydrated cement paste and can be considered as material properties. Microcracking is an apparent creep mechanism that can also contribute to the observed deformation and is responsible of the permanent deformation. Under high loading level, microcracks, initiated by the local stress, develop and interact with the viscoelasticity [1]. Then a deviation of the linearity of the mechanical response may occur and is manifested by tertiary creep [2,3].
The study of creep in tension has shown different effect on the behaviour of concrete with sometimes some contradiction. On one hand, creep may relax 1 internal tensile stresses generated by restrained shrinkage by increasing the deformation capacity to the rupture and consequently reducing the risk of potential cracking in concrete [4,5]. On the other hand, the principal mechanism of tensile creep is due to the microcracks development which could be responsible of the decrease of the residual strength and the modification of concrete properties [6,7]. Many researchers tried to quantify the effect of tensile creep on the behaviour of concrete mainly by measuring the residual strength [8][9][10][11][12][13]. A recent study conducted by the authors shows, with the acoustic emission (AE) technique, a more brittle behaviour and a decrease in the fracture process zone (FPZ) in specimens subjected to flexural creep [7]. But what is the reason of this brittleness after creep? And how do micro-cracks develop in the microstructure during creep?
The objective of this paper is to suggest an assessment of the damage mechanisms occurring during the different phases of creep. To achieve this, an experimental investigation is proposed on beams loaded with flexural creep at high stress levels. Damage evolution under creep is assessed by using the AE technique. This non-destructive technique proves to be very effective, especially to check and measure micro-cracking that takes place inside a structure under mechanical loading and it is particularly recommended to detecting and localizing cracks in concrete [14][15][16][17][18]. In our study, basic and desiccation creep were monitored at 70 and 85 % of the maximal strength. The results aim to investigate the ranges of variation of the time response due to creep damage coupled effects.
First of all, the materials and the experimental methods are presented. Then, the flexural creep tests are analyzed. Finally, the characterization of the damage evolution during basic and desiccation creep is suggested by using the AE method. Concrete specimens were mixed with Portland cement CPA-CEMII 42.5, crushed limestone aggregate distributed in fine sand with a maximum size of 5 mm and crushed gravel of size 5-12.5 mm. A superplasticizer agent, based on modified polycarboxylic ether polymers, has been added for the workability. Table 1 shows the mix quantities of constituent materials. This mixture is characterized by a water-to-cement (W/C) ratio of 0.56 and a slump of 70 mm. The proportioning of the cement paste, sand and coarse aggregates were kept constant throughout the program.
For the flexural test, 800 9 200 9 100 mm 3 (L 9 h 9 b) concrete beams were prepared with an effective span (S) equal to 600 mm. The fresh concrete was poured into beam moulds. A plate vibrator was used to compact the concrete in two layers. Then specimens were covered with a thin sheet of plastic to prevent water loss and were maintained in a climatic chamber at a temperature of 20°C and a relative humidity (RH) of 95 %. 24 h after casting, specimens were stripped off from the moulds and kept for curing in lime water, under a temperature condition of 20°C. Before creep tests, specimens were taken out from the curing tanks and a central notch was formed using a diamond saw cut, with a notch-to-depth ratio of 0.2 (a 0 = h/5).

Procedure for the three-point bending test
Three point bending fracture tests were realized to determine the maximum load (F max ) so we could load the specimens in creep. The fracture test uses a loadcontrolled universal testing machine as per RILEM-TMC 50 recommendations [19]. The load was applied with a slow rate of 0.3 lm/s, such that the peak load was reached at about 2 min. The averaged maximal strength measured on three specimens is 9.9 kN at 1 month and 10.8 kN at 8 months.
Flexural creep tests were then performed on frames with a capacity ranging from 5 to 50 kN. The frames were placed in a climate controlled chamber at 50 % RH and temperature of 20°C. The load is applied by gravity with a weight and counterweight system, which enables a fine tuning of the load. The displacement was measured at midspan on notched specimens ( Fig. 1). For the basic flexural creep tests, the exchange of moisture was prevented by a double layer of self-adhesive aluminium paper. Hence basic creep displacement was considered only. Two different tests were realized. First of all, basicdesiccation creep tests concerning beams subjected to basic creep and followed by desiccation creep at 70 and 85 % of F max are realized on specimens at the ages of 1 and 8 months. Those tests allow having a clear idea on the difference between basic and desiccation creep by eliminating the differences between beams due to concrete heterogeneity. Specimens were continuously monitored with the AE technique during basic and desiccation creep tests till the rupture. Second of all, desiccation creep tests concerning beams subjected to desiccation at 85 and 70 % of F max were realized and full AE waveforms were recorded up to failure.

Acoustic emission (AE) technique
The AE system comprised of an eight channel AE Win system, a general-purpose interface bus (PCI-DISP4) and a PC for data storage analysis. Eight piezoelectric transducers (resonant frequency of 150 kHz) were used to convert the mechanical waves to electrical signals. Transducers were placed around the expected location of the FPZ to minimize errors in the AE event localization program [20]. They were placed in a 3D parallelepiped position on both sides of the specimen, with silicon grease as the coupling aging (Fig. 2). The recorded AE amplitudes range from 0 to 100 dB. The detected signals were amplified with a 40 dB gain differential amplifier. In order to overcome the background noise, the signal detection threshold was set at a value of about 35 dB (value adjusted before every test) slightly above the measured background noise [20]. The acquisition system was calibrated before each test using a pencil lead break procedure HSU-NIELSEN (Norme NF EN 1330). The effective velocity and the attenuation of acoustic waves were also calculated. For this analysis, the effective velocity was assumed to be a constant for the analysis of AE source locations even though there may be some variability depending on the wave propagation path. The effective velocity was assumed to be 3,800 m/s. In order to eliminate mechanical and electro-magnetic disturbances, a low-pass filter with a cut-off frequency of 20 kHz, and a high-pass filter with a cut-off frequency of 400 kHz were used. Signal descriptors such as rise time, counts, energy, duration, amplitude, average frequency and counts to peak were captured and calculated by AEwin system. Each waveform was digitized and stored. The descriptors were further analyzed and evaluated with the software Noesis.
During the formation of a microcrack, energy is emitted as an elastic wave and propagates from the crack location to the AE transducers at the specimen surface. The locations of the AE sources are evaluated based on the arrival times of the first wave at each transducer and their respective velocity in concrete specimen. Once the arrival time is picked, the leastsquare method is used to assess the event location. The accuracy of the source location was estimated by applying the pencil lead fracture at a known location on the specimens. The location resolution was estimated to be ±5m m . the first days of loading (primary creep) and then stabilizes (secondary creep). The larger the applied stress, the more important are the kinetics and the magnitude of creep displacement. In addition, the ageing results in a decrease of the time-dependent displacement. When subjected to desiccation, creep displacement increases quickly and the beams loaded at 85 % failed few hours later while the beams loaded at 70 % failed after few days. The kinetic of the displacement during desiccation can be divided in two phases. During the first phase, the kinetic is very important and corresponds to the departure of water at the surface and the important desiccation due to water redistribution. The second part presents a lower kinetic in correlation with a more stable shrinkage deformation due to the departure of water inside the beam. Under loading, the bottom part of the beam is under tension and the top part is under compression. So, the microcracked layer due to desiccation in the bottom part of the beam is more extended and tends to loose its residual strength while the upper part of the specimen is forced to contract. This compressed part of the beam has a shrinkage rate more important than the part in tension. The increment of hardening becomes distributed asymmetrically and the neutral axis move upward causing an additional curvature [21,22].

Desiccation creep tests
Creep displacements obtained with the desiccation creep tests are plotted in Fig. 4. Specimens, loaded at the age of 8 months, failed after 1 day at 85 % and 3 days at 70 %. In fact, microcracking initiated due to the applied constant load begins to growth and to form a crack path [6,[23][24][25].
These tests showed that coupling between creep and damage seems to be more sensible to desiccation. In the following, the AE method has been used in order to understand the phenomena occurred in specimens.

Exploitation of the AE method to identify the creep-damage coupling in a basic-desiccation creep test
The analysis of the AE data permits real time detection and monitoring of active defects and can reflect the damage mechanisms of the specimen during creep. The combined basic-desiccation creep test realised on the beam aged of 8 months and loaded at 70 % of F max is analysed in the following. The analysis is made in two steps: the localization of AE events and then the classification of AE data.  During basic creep, events are arbitrarily distributed and diffused along the length (x, y) and the depth (y, z) of the specimen (Fig. 5a). During desiccation, the number of AE events increases with a higher rate and more energetic events, especially at the surfaces subjected to drying (Fig. 5b). Those events are highly dependent on desiccation. In fact, the non uniform desiccation (humidity gradient) induces a non uniform shrinkage in the specimen and thus presents structural consequences [26,27]. Then, events begin to localize at the front of the notch in the zone of the maximum tensile stress. As the average stress along the ligament surface is lower than the stress in front of the crack, microcracks relax the stress in front of the FPZ by the creation of new surfaces. Then, events follow a conical progress before the total failure where there is an emission of high amplitude and energetic signals (Fig. 5c). Those results allow us to understand the influence of creep on the brittleness of concrete observed during the failure of beams subjected to creep [7,28]. Note here that the relative kinetics of acoustic waves does not present an important variation during the test.

Correlation between creep displacement and AE parameters
The correlation between creep displacement and the characteristics of AE signals collected during creep is shown in Fig. 6. The AE activity is important during primary creep with the emission of high amplitude signals and then decreases and stabilizes during secondary creep. At the moment where the beam was subjected to desiccation, the number of AE hits increases quickly with the emission of high amplitude signals, then decreases progressively in correlation with shrinkage. The cumulated AE energy follows the same evolution and gives informations on the crack initiation that progress until the failure. Thus, it could be related to the fracture energy measured on a global scale. This finding strengthens the presumption that the acoustic events recorded during creep are related to the creation of micro-cracks or in other terms the damage occurring inside the material under creep.

Multivariable data clustering of AE signals
The quantitative understanding of the physical processes and the microstructural phenomena that control the fracture behaviour on the macroscopic scale is poor. During the last years, quantitative evaluation of fracture processes in concrete consisted in evaluating the different mode of failure and stress fields based on moment tensors [29][30][31] and some AE indices as the average frequency and the RA value which is defined by the rise time to the peak amplitude ratio [32]. It appears then necessary to take the analysis further to obtain information about the physical mechanisms, origin of the AE signatures. For this, a multi variable analysis of the recorded acoustic signals is proposed to discriminate the damage mechanisms in the material according to the typical AE signals and their apparition chronology.
For the classification process of the monitored AE data under creep, the non supervised method K-means associated with a principal component analysis (PCA) and the dendrogram are proposed [33]. The K-means method allows obtaining a non-supervised classification in n class representative of the n damage mechanisms in the case of multidimensional data 6 [34]. The PCA method is achieved in order to improve the visualisation of the classification result by reducing the dimension of the data [35]. In the nonsupervised method each signal can be associated to a pattern composed of multiple relevant features extracted from the random AE waveforms (amplitude, energy, rising time, average frequency…). Those parameters can be correlated and consequently redundant. It is then necessary to choose those descriptors wisely. The parameters were classified hierarchically with the dendrogram (Fig. 7) which exhibits the correlation level among the AE features. The correlation level was set to 0.9 and the descriptors were normalized in the interval of [-1; 1] to impose an equivalent weight factor to each AE component. The descriptors used are the energy, the absolute energy, the amplitude, the rise time, the counts, the counts to peak, the average frequency and the duration of the signals.
The results of the K-means method are presented in Fig. 8 in 2D in function of the first and second principal components that represent the most important variance of AE parameters. Two clusters are distinguished for basic creep and three for desiccation creep. The clusters are well separated and discriminated.
In the case of basic creep, the first cluster corresponds to signals of weak energy while the second cluster corresponds to signals of higher energy (Fig. 9). For desiccation creep, the same behaviour is observed for the clusters 1 and 2 and the additional cluster 3 is characterized by signals of very weak energy. The apparition chronology of these clusters shows that the first is the most distinguished damage mechanism during basic creep and involves much more numerous AE hits than the second class (Fig. 10). During desiccation creep, the same trend is observed for the first two clusters and the AE hits distribution of the third cluster appears the most important mainly at the beginning of desiccation and decreases with time. In addition, the number of AE hits for the clusters 1 and 2 increases in desiccation in comparison with basic creep.
The number of hits by amplitude recorded was averaged to create an experimental distribution of the AE hits amplitude for each cluster and was fitted with a statistical Laplace-Gauss model. The Laplace-Gauss model was characterized by two parameters: the mode, which is the population mean and the range which represents the full width at half maximum.
where f x ðÞ is the statistical variation of the population, r the population standard deviation, x the studied parameter and m the population mean. Figure 11 shows the experimental distribution and the corresponding statistical law of the AE hits amplitude for each class. The mode of the AE hits amplitude distribution for the first cluster is 42 dB and the range is between 36 and 47 dB and can be associated to microcracking at the matrix-aggregate interface [36]. For the second class, the mode is 50 dB and the range is between 42 and 59 dB and can be associated to micro-cracking in the matrix [36]. For the third cluster, the mode is 37 dB and the range is between 35 and 41 dB. Based on the variation of the AE parameters, this cluster could correspond to signals due to drying as liquid transfer in concrete [37,38] and cavitation [39]. Note that the differences between ranges of amplitude of classes obtained here could be different for others specimen geometries and recording system parameters. The ranges have to be considered as relative differences. Through this approach, we have shown that it is possible, using the AE method, to identify the most critical damage mechanisms leading to the final failure of concrete. In order to study the damage evolution during the three creep phases at the micro-structural level and more particularly tertiary creep, the AE technique was also used during desiccation creep tests. The possibility of assessing time to failure of the tested beams from AE is also investigated.  Absolute energy (aJ) Fig. 12 Correlation between the creep kinetic and the AE hits amplitude (left); correlation between the cumulated AE energy and the distribution of the AE hits (right) was removed and the AE activity was followed during the three distinct phases of creep corresponding to the evolution of creep displacement into three regimes: primary creep, which corresponds to a fast decrease of strain kinetic under the initial load, followed by secondary creep, which corresponds to a quasiconstant strain kinetic, and tertiary creep in which the strain kinetic increases quickly leading to the global failure of the beams. Those phases generate different signals covering different ranges of amplitude and corresponding to different damage mechanisms.
The AE activity is important during primary creep with AE hits of high amplitude and an important emission of AE energy (Fig. 12). The rate decreases in correlation with the rate of creep displacement. During this phase, the events are arbitrary distributed especially in the tension zone (Fig. 13a) and may correspond to the initiation and the development of microcracks inside the material as other physical mechanisms responsible of creep as water and stress redistribution in the beams and consequently microcracking.
During secondary creep, the rate of the AE activity is quasi-constant with a stable evolution of AE energy (Fig. 12). The number of events continues to increase with different energetic value near the notch (Fig. 13b). This phase corresponds to the apparition of a new damage mechanism due to the extension and the propagation of microcracking. Stresses are also generated by the deformation incompatibility between the aggregate and the cement paste [40,41]. This could be seen on the localization map which presents events of different energy and which corresponds to different damage mechanisms as micro-cracks at the interface between the matrix and aggregate and in the matrix [42].
During the last phase, creep evolves toward the tertiary creep regime where the strain rate accelerates up to failure. The AE activity increases quickly with the emission of very energetic signals. This phase corresponds to the coalescence and the fast propagation of microcracks generating a localized crack and The amplitude of the AE signals in this phase covers different ranges and reaches sometimes 100 dB at the failure where the events begin to concentrate in the cracking zone to create finally a macroscopic crack (Fig. 13c).
The stress concentration and redistribution are responsible of the failure and depend highly on the rate of loading and the loading condition. The rate of stress modifies the crack development and causes a slow and stable increase of microcracks until the unstable condition is reached during tertiary creep. This structural damage can be correlated to the evolution of microcracks or hits by relating the rate of the cumulated number of AE hits (N) and the number obtained at the end of the test (N max ), corresponding to the total failure where the scalar damage value is equal to 1 [43]: where N max = 3,425 and N max = 5,900 for the beams loaded at 85 and 70 % respectively. Figure 14 shows the evolution of the damage coefficient during flexural creep tests at 70 and 85 %. The rate of damage measured for the creep at 85 % is more important in correlation with the rate of loading and the kinetics of creep displacement. Before the failure, creep displacement increases with an exponential function and residual life-time duration can be then estimated. This damage accumulation evolves as a bathtub-shaped curve and can be described using a Weibull function [44]. That suggests a method to predict the failure by following the AE activity during creep and allows estimating the degree of concrete deterioration at an early stage of the deformation before the macrocrack formation. But it needs more creep tests with different specimen sizes and loading conditions.

Conclusion
An experimental investigation concerning the use of the AE method to characterize local damage and to analyze the physical mechanisms underlying creep of concrete has been carried out. A good correlation was observed between creep displacement and the variation of the AE parameters. The coupling between creep and damage seems to be more important in desiccation. As a part of the investigation, quantitative analysis of the AE data was applied and characteristics of individual microcracks were evaluated and associated to two clusters for basic creep and three clusters for desiccation creep. The differences of the AE activity during the three regimes of creep displacement were identified. The state of damage increases with the rate of loading and based on this study we could have sufficient data in order to predict the non linear creep and the failure of concrete. In order to have more information on the microstructural effect and the heterogeneity of concrete, similar creep tests will be also realized on mortar beams and monitored with the AE technique. Those tests will provide additional information on the time dependency of each identified damage mechanism and the effect of aggregate on the fracture behaviour. The possibility of combining the multivariable data clustering with the moment tensor will be also studied.