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Article Dans Une Revue The European Physical Journal D : Atomic, molecular, optical and plasma physics Année : 2015

Non-markovian polariton dynamics in organic strong coupling

Résumé

Strongly coupled organic systems are characterized by unusually large Rabi splitting, even in the vacuum state. They show the counter-intuitive feature of a lifetime of the lower polariton state longer than for all other excited states. Here we build up a new theoretical framework to understand the dynamics of such coupled system. In particular, we show that the non-Markovian character of the relaxation of the dressed organic system explains the long lifetime of the lower polariton state.

Dates et versions

hal-00850074 , version 1 (02-08-2013)

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Antoine Canaguier-Durand, Cyriaque Genet, Astrid Lambrecht, Thomas W. Ebbesen, Serge Reynaud. Non-markovian polariton dynamics in organic strong coupling. The European Physical Journal D : Atomic, molecular, optical and plasma physics, 2015, 69, pp.24. ⟨10.1140/epjd/e2014-50539-x⟩. ⟨hal-00850074⟩
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