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Article Dans Une Revue Energy & Fuels Année : 2012

Hydrogen Production by Homogeneous Partial Oxidation of Propane

Résumé

A kinetic study of the partial oxidation of propane was performed in a jet stirred reactor. The main goal of this study was to establish a detailed homogeneous mechanism of this reaction and explore the capability to produce H2 and olefins. Various operating parameters are modified: temperature, residence time, and O2/C3H8 ratio. The mechanism was validated by comparing experimental and simulated results. A different behavior was observed depending on the temperature. At 600 °C, the mechanism contains both an oxidation and a pyrolytic path. The main products are H2, C2H4, CH4, CO, and O2. At 800 °C, the mechanism mostly contains a pyrolytic path. The main products are H2 and CO.
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Dates et versions

hal-00693221 , version 1 (02-05-2012)

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C. Hognon, Y. Simon, P.M. Marquaire. Hydrogen Production by Homogeneous Partial Oxidation of Propane. Energy & Fuels, 2012, 26 ((3)), pp.1496-1508. ⟨10.1021/ef201938t⟩. ⟨hal-00693221⟩
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