Tight-binding calculations of image charge effects in colloidal nanoscale platelets of CdSe

Abstract : CdSe nanoplatelets show perfectly quantized thicknesses of few monolayers. They present a situation of extreme, yet well de ned quantum con nement. Due to large dielectric contrast between the semiconductor and its ligand environment, interaction between carriers and their dielectric images strongly renormalize bare single particle states. We discuss the electronic properties of this original system in an advanced tight-binding model, and show that Coulomb interactions, including self-energy corrections and enhanced electron-hole interaction, lead to exciton binding energies up to several hundred meVs.
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Ramzi Benchamekh, Nikolay A. Gippius, Jacky Even, Mikhail Nestoklon, Jean-Marc Jancu, et al.. Tight-binding calculations of image charge effects in colloidal nanoscale platelets of CdSe. Physical Review B : Condensed matter and materials physics, American Physical Society, 2014, 89 (3), pp.035307. ⟨10.1103/PhysRevB.89.035307⟩. ⟨hal-00942566⟩

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