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Physical Review Letters 109 (2012) 093902
Wide-Field Vibrational Phase Imaging
Pascal Berto 1, David Gachet 2, Pierre Bon 1, Serge Monneret 1, Herve Rigneault 1
(28/08/2012)

We propose and implement a wide-field microscopy method to retrieve the real and imaginary part of a field emitted by coherent and resonant molecular scatterers. The technique is based on wave-front sensing and does not require the use of any reference beam. We exemplify its ability in wide-field coherent anti- Stokes Raman scattering imaging and retrieve the complex anti-Stokes field while spectrally scanning a molecular vibrational resonance. This approach gives access to the background-free Raman spectrum of the targeted molecular bond.
1 :  Institut FRESNEL (IF)
CNRS : UMR7249 – Ecole Centrale de Marseille – Aix-Marseille Université - AMU
2 :  Centre Interdisciplinaire de Nanosciences de Marseille (CINaM)
CNRS : UPR3118
MOSAIC
Sciences de l'ingénieur/Optique / photonique