MIPAS detects Antarctic stratospheric belt of NAT PSCs caused by mountain waves

M. Höpfner (1) , N. Larsen (2) , R. Spang (3) , B. P. Luo (4) , J. Ma (5) , S. H. Svendsen (2) , S. D. Eckermann (6) , B. Knudsen (2) , P. Massoli (7) , F. Cairo (7) , G. Stiller (1) , T. V. Clarmann (1) , H. Fischer (1)

1 Forschungszentrum Karlsruhe
2 DMI - Danish Meteorological Institute
3 FZJ - Forschungszentrum Jülich GmbH | Centre de recherche de Jülich | Jülich Research Centre
4 Institut für Atmosphäre und Klima [Zürich]
5 Computational Physics, Inc.
6 E. O. Hulburt Center for Space Research
7 CNR - National Research Council of Italy | Consiglio Nazionale delle Ricerche

Space borne infrared limb emission measurements by the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) reveal the formation of a belt of polar stratospheric clouds (PSCs) of nitric acid trihydrate (NAT) particles over Antarctica in mid-June 2003. By mesoscale microphysical simulations we show that this sudden onset of NAT PSCs was caused by heterogeneous nucleation on ice in the cooling phases of large-amplitude stratospheric mountain waves over the Antarctic Peninsula and the Ellsworth Mountains. MIPAS observations of PSCs before this event show no indication for the presence of NAT clouds with volume densities larger than about 0.3 ?m³/cm³ and radii smaller than 3 ?m, but are consistent with supercooled droplets of ternary H₂SO₄/HNO₃/H₂O solution (STS). Simulations indicate that homogeneous surface nucleation rates have to be reduced by three orders of magnitude to comply with the observations.

Domaines: Océan, Atmosphère

M. Höpfner, N. Larsen, R. Spang, B. P. Luo, J. Ma, et al.. MIPAS detects Antarctic stratospheric belt of NAT PSCs caused by mountain waves. Atmospheric Chemistry and Physics Discussions, 2005, 5 (5), pp.10723-10745. ⟨hal-00301880⟩