Size distribution and hygroscopic properties of aerosol particles from dry-season biomass burning in Amazonia
Résumé
Aerosol particle number size distributions and hygroscopic properties were measured at a pasture site in the southwestern Amazon region (Rondonia). The measurements were performed 11 September?14 November 2002 as part of LBA-SMOCC (Large scale Biosphere atmosphere experiment in Amazonia ? SMOke aerosols, Clouds, rainfall and Climate), and cover the later part of the dry season (with heavy biomass burning), a transition period, and the onset of the wet period.
Particle number size distributions were measured with a DMPS (Differential Mobility Particle Sizer, 3?850 nm) and an APS (Aerodynamic Particle Sizer), extending the distributions up to 3.3 µm in diameter. An H-TDMA (Hygroscopic Tandem Differential Mobility Analyzer) measured the hygroscopic diameter growth factors (Gf) at 90% relative humidity (RH), for particles with dry diameters (dp) between 20?440 nm, and at several occasions RH scans (30?90% RH) were performed for 165 nm particles. These data provide the most extensive characterization of Amazonian biomass burning aerosol, with respect to particle number size distributions and hygroscopic properties, presented until now. The evolution of the convective boundary layer over the course of the day causes a distinct diel variation in the aerosol physical properties, which was used to get information about the properties of the aerosol at higher altitudes.
The number size distributions averaged over the three time periods showed three modes; a nucleation mode with count median diameters (CMD) of ~12 nm, an Aitken mode (CMD = 61?92 nm) and an accumulation mode (CMD = 128?190 nm). The two larger modes were shifted towards larger CMD with increasing influence from biomass burning.
Particle number size distributions were measured with a DMPS (Differential Mobility Particle Sizer, 3?850 nm) and an APS (Aerodynamic Particle Sizer), extending the distributions up to 3.3 µm in diameter. An H-TDMA (Hygroscopic Tandem Differential Mobility Analyzer) measured the hygroscopic diameter growth factors (Gf) at 90% relative humidity (RH), for particles with dry diameters (dp) between 20?440 nm, and at several occasions RH scans (30?90% RH) were performed for 165 nm particles. These data provide the most extensive characterization of Amazonian biomass burning aerosol, with respect to particle number size distributions and hygroscopic properties, presented until now. The evolution of the convective boundary layer over the course of the day causes a distinct diel variation in the aerosol physical properties, which was used to get information about the properties of the aerosol at higher altitudes.
The number size distributions averaged over the three time periods showed three modes; a nucleation mode with count median diameters (CMD) of ~12 nm, an Aitken mode (CMD = 61?92 nm) and an accumulation mode (CMD = 128?190 nm). The two larger modes were shifted towards larger CMD with increasing influence from biomass burning.
Domaines
Océan, Atmosphère
Origine : Accord explicite pour ce dépôt
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