High-frequency acoustic modes in silica via ultrafast optical techniques
Résumé
We use the advent of reliable ultrafast optical techniques to explore acoustic modes in glasses in the difficult but crucial frequency region between around 0.1 and 1 THz. Brillouin scattering of light allows to measure velocity and absorption of sound up to frequencies around 100 GHz and coherent inelastic x-ray scattering (IXS) is limited to frequencies larger than 1 THz. A rather universal property of glasses is that a large excess of modes exists, with a maximum density of states near 1 THz, forming the so-called boson peak. The acoustic modes are expected to be strongly affected as their frequency nears the boson peak. The onset of this effect, which is expected to be dominant in the 0.5 to 1 THz range, is observed here for the first time in v-SiO2 as a function of temperature.