Atomic-like spin noise in solid-state demonstrated with manganese in cadmium telluride

Steeve Cronenberger (1) , Denis Scalbert (1) , David Ferrand (2) , Hervé Boukari (2) , Joël Cibert (2)

1 L2C - Laboratoire Charles Coulomb
2 NEEL - NPSC - Nanophysique et Semiconducteurs

Spin noise spectroscopy is an optical technique which can probe spin resonances non-perturbatively. First applied to atomic vapours, it revealed detailed information about nuclear magnetism and the hyperfine interaction. In solids, this approach has been limited to carriers in semiconductor heterostructures. Here we show that atomic-like spin fluctuations of Mn ions diluted in CdT e (bulk and quantum wells) can be detected through the Kerr rotation associated to excitonic transitions. Zeeman transitions within and between hyperfine multiplets are clearly observed in zero and small magnetic fields and reveal the local symmetry because of crystal field and strain. The linewidths of these resonances are close to the dipolar limit. The sensitivity is high enough to open the way towards the detection of a few spins in systems where the decoherence due to nuclear spins can be suppressed by isotopic enrichment, and towards spin resonance microscopy with important applications in biology and materials science.

Mots clés: manganese; spin noise spectroscopy

Domaines: Matière Condensée [cond-mat]

Steeve Cronenberger, Denis Scalbert, David Ferrand, Hervé Boukari, Joël Cibert. Atomic-like spin noise in solid-state demonstrated with manganese in cadmium telluride. Nature Communications, 2015, 6, pp.8121. ⟨10.1038/ncomms9121⟩. ⟨hal-01216561⟩